Best known as author of the "Smyth Report," the official government report on the development of the atomic bomb, Henry DeWolf Smyth had a long and varied career as a physicist, diplomat, instructor, policy maker, and administrator. Taking leave from his position with the Physics Department at Princeton, Smyth began work on the Uranium committee of the National Defense Research Committee in 1940, serving as a consultant on the Manhattan Project from 1943-1945. Although he returned to Princeton after the war, Smyth left academia to become Commissioner of the U.S. Atomic Energy Commission (AEC) from 1949 to 1954, and he subsequently served as U.S. Representative to the International Atomic Energy Agency (IAEA), from 1961 to 1970. The Smyth Papers (1885-1987) contain correspondence, subject files, speeches, manuscripts of unpublished and published works, reprints and printed publications, scientific class notes and papers, newspaper clippings, photographs, and memorabilia which document Smyth's career as a physicist and statesman. The bulk of the collection dates from approximately 1944 to 1970, the most active and influential years of his career, providing good documentation of his work on the Manhattan Project and the Smyth Report, and his involvement with the U.S. Atomic Energy Commission and the International Atomic Energy Commission.

A gifted mathematician, Polish-born Stanislaw Ulam made contributions to set theory, topology, mathematical logic, and number theory, but is most widely remembered for his work in fostering the technical development of thermonuclear weapons. He was associated with Los Alamos Scientific Laboratories for most of the years between 1943 and 1965, and thereafter with the University of Colorado. These papers include personal and professional correspondence, manuscripts of both published and unpublished works, and memorabilia.

John Archibald Wheeler (1911-2008) was a leading theoretical physicist of the twentieth century, contributing particularly to the fields of general relativity, gravitation, and quantum mechanics. Wheeler was a pioneer in the study of black holes, celestial phenomena which he named. (He had a penchant for creating new terms in physics, and is credited with naming other phenomena such as geons, wormholes, and quantum foam.) Wheeler is also known for his work in atomic and nuclear physics. In 1939, he and Niels Bohr co-authored a paper that gave the basis for recognizing that Uranium 235 and Plutonium 239 are highly fissile, a milestone in the understanding of atomic energy. Wheeler believed in the importance of public service, assisting in the U.S. war effort to develop the atomic and hydrogen bombs, and served as a scientific advisor to numerous government agencies. During a prolific academic career that spanned seventy years, Wheeler taught physics to thousands of undergraduate students at Princeton University and the University of Texas, and mentored more than fifty Ph.D. students. The Wheeler Papers provide an extensive look into the expansive career of John Archibald Wheeler, the pioneering and award-winning theoretical physicist. Comprised of 150 linear feet, this large collection contains a wide array of materials including correspondence, subject files, manuscripts by Wheeler, papers by colleagues and students, research notes and notebooks, photographs, awards, and audiovisual materials. The collection provides much insight in to Wheeler's lengthy career as a scientist, scholar, and teacher. The bulk of the material is from the 1950s to the 1990s and covers the wide scope of his professional endeavors, from his teaching at Princeton University and the University of Texas, to his many publications, to his consultation work with government agencies, industry, and atomic energy projects, to his numerous public talks and lectures.

Primary source materials for the history of quantum physics in the twentieth century, collected under the auspices of the American Philosophical Society and the American Physical Society, with a grant from the National Science Foundation.